全文获取类型
收费全文 | 17061篇 |
免费 | 156篇 |
国内免费 | 121篇 |
专业分类
安全科学 | 366篇 |
废物处理 | 697篇 |
环保管理 | 1985篇 |
综合类 | 3748篇 |
基础理论 | 3847篇 |
环境理论 | 9篇 |
污染及防治 | 4409篇 |
评价与监测 | 1130篇 |
社会与环境 | 1096篇 |
灾害及防治 | 51篇 |
出版年
2022年 | 137篇 |
2021年 | 152篇 |
2019年 | 123篇 |
2018年 | 212篇 |
2017年 | 216篇 |
2016年 | 358篇 |
2015年 | 284篇 |
2014年 | 434篇 |
2013年 | 1224篇 |
2012年 | 491篇 |
2011年 | 688篇 |
2010年 | 529篇 |
2009年 | 606篇 |
2008年 | 709篇 |
2007年 | 733篇 |
2006年 | 670篇 |
2005年 | 545篇 |
2004年 | 564篇 |
2003年 | 547篇 |
2002年 | 533篇 |
2001年 | 639篇 |
2000年 | 398篇 |
1999年 | 303篇 |
1998年 | 193篇 |
1997年 | 210篇 |
1996年 | 229篇 |
1995年 | 237篇 |
1994年 | 239篇 |
1993年 | 219篇 |
1992年 | 198篇 |
1991年 | 209篇 |
1990年 | 200篇 |
1989年 | 171篇 |
1988年 | 168篇 |
1987年 | 154篇 |
1986年 | 155篇 |
1985年 | 148篇 |
1984年 | 169篇 |
1983年 | 169篇 |
1982年 | 173篇 |
1981年 | 144篇 |
1980年 | 132篇 |
1979年 | 123篇 |
1978年 | 134篇 |
1977年 | 117篇 |
1976年 | 104篇 |
1975年 | 108篇 |
1974年 | 118篇 |
1971年 | 98篇 |
1967年 | 101篇 |
排序方式: 共有10000条查询结果,搜索用时 406 毫秒
991.
N. Mithil Kumar K. Varaprasad G. Ramachandra Reddy G. Siva Mohan Reddy Y. Sivabharathi G. Venkata Subba Reddy S. Venkata Naidu 《Journal of Polymers and the Environment》2011,19(1):225-229
Synthesis and characterization of novel biodegradable, water soluble and optically active DL-malic acid (DMA) and citric acid
(CA) copolymers were studied for possible use as antibacterial agents. The copolymers were synthesized by direct bulk melt
condensation in the absence of a catalyst above 150 °C. Characterization of obtained copolymers was carried out with the help
of infrared absorption spectra, differential scanning calorimetry and thermo gravimetric analysis. The antibacterial activity
of copolymers against bacteria was investigated. The results obtained shows the above copolymers possess a broad wound dressing
activity against different types of bacteria and may be useful as antibacterial agents. 相似文献
992.
Caricasole P Provenzano MR Hatcher PG Senesi N 《Waste management (New York, N.Y.)》2011,31(3):411-415
In this paper, the evolution of organic matter (OM) during composting of different mixtures of various organic wastes was assessed by means of chemical analyses and CPMAS 13C NMR spectroscopy measured during composting. The trends of temperatures and C/N ratios supported the correct evolution of the processes. The CPMAS 13C NMR spectra of all composting substrates indicated a reduction in carbohydrates and an increase in aromatic, phenolic, carboxylic and carbonylic C which suggested a preference by microorganisms for easily degradable C molecules. The presence of hardly degradable pine needles in one of the substrates accounted for the lowest increase in alkyl C and the lowest reduction in carbohydrates and carboxyl C as opposite to another substrate characterized by the presence of a highly degradable material such as spent yeast from beer production, which showed the highest increase of the alkyl C/O-alkyl C ratio. The highest increase of COOH deriving by the oxidative degradation of cellulose was shown by a substrate composed by about 50% of plant residues. The smallest increases in alkyl C/O-alkyl C ratio and in polysaccharides were associated to the degradation of proteins and lipids which are major components of sewage sludge. Results obtained were related to the different composition of fresh organic substrates and provided evidence of different OM evolution patterns as a function of the initial substrate composition. 相似文献
993.
The results are presented that have been obtained during long-term studies (1991–2009) on the efficiency of natural reproduction
of the beluga, Russian sturgeon, stellate sturgeon, and sterlet in different spawning zones of the Volga. The influence of
major environmental factors on the formation of the offspring of these fishes is analyzed. It is shown that the productivity
of Volga spawning grounds varies depending on the river flow volume during spring floods and the abundance of active spawners.
Practical recommendations are proposed for enhancing sturgeon reproduction in the Volga. 相似文献
994.
J. Gasperi C. Sebastian V. Ruban M. Delamain S. Percot L. Wiest C. Mirande E. Caupos D. Demare M. Diallo Kessoo Kessoo M. Saad J. J. Schwartz P. Dubois C. Fratta H. Wolff R. Moilleron G. Chebbo C. Cren M. Millet S. Barraud M. C. Gromaire 《Environmental science and pollution research international》2014,21(8):5267-5281
This study aimed at: (a) providing information on the occurrence and concentration ranges in urban stormwater for a wide array of pollutants (n?=?77); (b) assessing whether despite the differences between various catchments (land use, climatic conditions, etc.), the trends in terms of contamination level are similar; and (c) analyzing the contribution of total atmospheric fallout (TAF) with respect to sources endogenous to this contamination. The studied contaminants include conventional stormwater contaminants (polycyclic aromatic hydrocarbons (PAHs), Zn, Cu, Pb, etc.), in addition to poorly or undocumented pollutants such as nonylphenol and octylphenol ethoxylates (NPnEO and OPnEO), bisphenol A (BPA), polybrominated diphenyl ethers (PBDEs), a wide variety of pesticides, and various metals of relevance (As, Ti, Sr, V). Sampling and analysis were performed using homogeneous methods on three urban catchments with different land use patterns located in three distinct French towns. For many of these pollutants, the results do not allow highlighting a significant difference in stormwater quality at the scale of the three urban catchments considered. Significant differences were, however, observed for several metals (As, Cr, Cu, Ni, Sr and Zn), PAHs, and PBDEs, though this assessment would need to be confirmed by further experiments. The pollutant distributions between dissolved and particulate phases were found to be similar across the three experimental sites, thus suggesting no site dependence. Lastly, the contributions of TAF to stormwater contamination for micropollutants were quite low. This finding held true not only for PAHs, as previously demonstrated in the literature, but also for a broader range of molecules such as BPA, NPnEO, OPnEO, and PBDEs, whose high local production is correlated with the leaching of urban surfaces, buildings, and vehicles. 相似文献
995.
Omar D. Cardona Mario G. Ordaz Mabel C. Marulanda Martha L. Carreño Alex H. Barbat 《Disasters》2010,34(4):1064-1083
The Disaster Deficit Index (DDI) measures macroeconomic and financial risk in a country according to possible catastrophic scenario events. Extreme disasters can generate financial deficit due to sudden and elevated need of resources to restore affected inventories. The DDI captures the relationship between the economic loss that a country could experience when a catastrophic event occurs and the availability of funds to address the situation. The proposed model utilises the procedures of the insurance industry in establishing probable losses, based on critical impacts during a given period of exposure; for economic resilience, the model allows one to calculate the country's financial ability to cope with a critical impact. There are limitations and costs associated with access to resources that one must consider as feasible values according to the country's macroeconomic and financial conditions. This paper presents the DDI model and the results of its application to 19 countries of the Americas and aims to guide governmental decision‐making in disaster risk reduction. 相似文献
996.
Fernando H. Pulgati Ricardo N. Ayup-Zouain Luiz Landau Jandyra M. G. Fachel 《Environmental monitoring and assessment》2010,167(1-4):79-89
This paper describes the use of Bayesian spatial models to develop the concept of a spatial–temporal mask for the purpose of identifying regions in which before and after drilling effects are most clearly defined and from which the consequences of exposure of macrofauna and meiofauna to the release of drilling discharges can be evaluated over time. To determine the effects of drilling fluids and drill-cuttings on the marine benthic community, it is essential to know not only where discharged materials ended up within the possible impact area, but also the chemical concentrations to which biota were exposed during and after drilling. Barium and light hydrocarbons were used as chemical tracers for water-based and non-aqueous-based fluids in a shallow water site in the Campos Basin, off the coast of Brazil. Since the site showed evidence of exposure to waste material from earlier drilling, the analysis needed to take into account the background concentrations of these compounds. Using the Bayesian models, concentrations at unsampled sites were predicted and regions altered and previously contaminated were identified. 相似文献
997.
The Water Framework Directive (WFD) has initiated a shift towards a targeted approach to implementation through its focus on river basin districts as management units and the natural ecological characteristics of waterbodies. Due to its role in eutrophication, phosphorus (P) has received considerable attention, resulting in a significant body of research, which now forms the evidence base for the programme of measures (POMs) adopted in WFD River Basin Management Plans (RBMP). Targeting POMs at critical sources areas (CSAs) of P could significantly improve environmental efficiency and cost effectiveness of proposed mitigation strategies. This paper summarises the progress made towards targeting mitigation measures at CSAs in Irish catchments. A review of current research highlights that knowledge related to P export at field scale is relatively comprehensive however; the availability of site-specific data and tools limits widespread identification of CSA at this scale. Increasing complexity of hydrological processes at larger scales limits accurate identification of CSA at catchment scale. Implementation of a tiered approach, using catchment scale tools in conjunction with field-by-field surveys could decrease uncertainty and provide a more practical and cost effective method of delineating CSA in a range of catchments. Despite scientific and practical uncertainties, development of a tiered CSA-based approach to assist in the development of supplementary measures would provide a means of developing catchment-specific and cost-effective programmes of measures for diffuse P. The paper presents a conceptual framework for such an approach, which would have particular relevance for the development of supplementary measures in High Status Waterbodies (HSW). The cost and resources necessary for implementation are justified based on HSWs' value as undisturbed reference condition ecosystems. 相似文献
998.
Karakaya and Sultansuyu Dam Lakes, located in the eastern part of Turkey, are important water sources, both for irrigation
and fishery. The main goal of the study was to investigate water qualities of dam lakes using a set of biomarkers in the fish
Cyprinus carpio. For this aim, field sample and laboratory-acclimated fish were compared to identify changes in selected biomarkers. The
activities of ethoxyresorufin-O-deethylase, glutathione S-transferase, glutathione reductase, and carboxylesterase were determined in liver samples. Also, plasma and liver lactate
dehydrogenase, aspartate aminotransferase, and alanine aminotransferase activities were assayed. Brain acetylcholinesterase
and carboxylesterase activities were also determined. The hepatosomatic index and condition factors were calculated. Plasma
vitellogenin assays were evaluated for the presence of xenoestrogen. Physicochemical values of water samples showed the existence
of eutrophication risk, and also, some chemicals in both lakes were determined to be over tolerable limits. The comparisons
of samples from both dam lake and laboratory-acclimated fish showed that the lakes may be at risk of pollution by some xenobiotics,
namely xenoestrogens and acetylcholinesterase-inhibiting agents. 相似文献
999.
Arruda-Neto JD Nieto L Righi H Cotta MA Carrer H Rodrigues TE Genofre GC 《Journal of environmental monitoring : JEM》2012,14(8):2108-2113
Persistent harmful scenarios associated with disposal of radioactive waste, high-background radiation areas and severe nuclear accidents are of great concern regarding consequences to both human health and the environment. Of particular concern is the extracellular DNA in aquatic environments contaminated by radiological substances. Strand breaks induced by radiation promote decrease in the transformation efficiency for extracellular DNA. The focus of this study is the quantification of DNA damage following long-term exposure (over one year) to low doses of natural uranium (an alpha particle emitter) to simulate natural conditions, since nothing is known about alpha radiation induced damage to extracellular DNA. A high-resolution Atomic Force Microscope was used to evaluate DNA fragments. Double-stranded plasmid pBS as a model for extracellular DNA was exposed to different amounts of natural uranium. It was demonstrated that low concentrations of U in water (50 to 150 ppm) produce appreciable numbers of double strand breaks, scaling with the square of the average doses. The importance of these findings for environment monitoring of radiological pollution is addressed. 相似文献
1000.
Priyanka A. Bedekar Rijuta G. Saratale Ganesh D. Saratale Sanjay P. Govindwar 《Environmental science and pollution research international》2014,21(18):11075-11085
Lysinibacillus sp. RGS degrades sulfonated azo dye Reactive Orange 16 (RO16) efficiently. Superoxide dismutase and catalase activity were tested to study the response of Lysinibacillus sp. RGS to the oxidative stress generated by RO16. The results demonstrated that oxidative stress enzymes not only protect the cell from oxidative stress but also has a probable role in decolorization along with an involvement of oxidoreductive enzymes. Formation of three different metabolites after degradation of RO16 has been confirmed by GC-MS analysis. FTIR analysis verified the degradation of functional groups of RO16, and HPTLC confirmed the removal of auxochrome group from the RO16 after degradation. Toxicity studies confirmed the genotoxic, cytotoxic, and phytotoxic nature of RO16 and the formation of less toxic products after the treatment of Lysinibacillus sp. RGS. Therefore, Lysinibacillus sp. RGS has a better perspective of bioremediation for textile wastewater treatment. 相似文献